The nonlinear absorption of Au–Ag nanoplanets made by Ar irradiation of bimetallic nanoclusters in silica has been experimentally investigated by means of the single beam z-scan technique. The measurements have been performed in the picoseconds regime in order to isolate the fast electronic contribution to the third-order nonlinearity. The results reveal large nonlinear absorption properties of these systems, characterized by the concomitance of saturable and reverse saturable absorption. A phenomenological expression has been developed to fit the z-scan curves and to quantitatively determine the nonlinear optical parameters.
Nonlinear optical properties of Au-Ag nanoplanets made by ion beam processing of bimetallic nanoclusters in silica.
CESCA, TIZIANA;PELLEGRINI, GIOVANNI;BELLO, VALENTINA;SCIAN, CARLO;MAZZOLDI, PAOLO;BATTAGLIN, GIANCARLO;MATTEI, GIOVANNI
2010
Abstract
The nonlinear absorption of Au–Ag nanoplanets made by Ar irradiation of bimetallic nanoclusters in silica has been experimentally investigated by means of the single beam z-scan technique. The measurements have been performed in the picoseconds regime in order to isolate the fast electronic contribution to the third-order nonlinearity. The results reveal large nonlinear absorption properties of these systems, characterized by the concomitance of saturable and reverse saturable absorption. A phenomenological expression has been developed to fit the z-scan curves and to quantitatively determine the nonlinear optical parameters.File in questo prodotto:
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